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- Poems (1853)
- Sonnets on the War (1855), co-authored with Sydney Thompson Dobell
- City Poems (1857)
- Edwin of Deira (1861)
- Dreamthorp: a Book of Essays written in the Country (1863)
- A Summer in Skye (1865), in 2 vols.
- Alfred Hagart's Household and Miss Dona M'Quarrie (1866), in 2 vols.
- Last Leaves (1868), edited with memoir by Patrick Proctor Alexander
- Poetical Works of Burns (1865), in 2 vols.
- Golden Leaves from the American Poets (1866)
Works about Smith
- The early years of Alexander Smith, poet and essayist (1869), by Thomas Brisbane