- active product in the atmosphere with those of the known radio-active
products of thorium and radium. A cursory examination of the facts at once shows that the radio-activity of the atmosphere is much more closely allied to effects produced by radium than to those due to thorium. The activity of the emanation released from well water, and also that sucked up from the earth, decays to half value in about 3·3 days, while the activity of the radium emanation decays to half value in an interval of 3·7 to 4 days. Considering the difficulty of making accurate determinations of these quantities, the rates of decay of the activity of the emanations from the earth and from radium agree within the limits of experimental error. A large number of observers have found that the radium emanation is present in the water of thermal springs and in the sediment deposited by them. Bumstead and Wheeler have shown that the emanation from the soil and surface water of New Haven is identical with that from radium. If the emanations from the earth and from radium are the same, the excited activities produced should have the same rate of decay. The emanation from well water in England approximately fulfils this condition (section 276), but an observation recorded by Ebert and Ewers (section 276) seems to show that the excited activity due to the emanation sucked up from the earth decays at a very slow rate compared with that due to radium.
Bumstead has given undoubted evidence that the thorium as well as the radium emanation is also present in the atmosphere at New Haven, while Dadourian has shown that it is emitted by New Haven soil. Blanc, and Elster and Geitel, have also found that thorium is present in the sediment from some thermal springs.
If the active matter in the atmosphere consists mainly of the radium emanation, the active deposit on a negatively charged wire, exposed in the open air, should initially consist of radium A, B and C. The curve of decay should be identical with the decay curve of the excited activity of radium, measured by the α rays, that is, there should be a rapid initial drop corresponding to the initial 3 minute change, then a slow rate of variation, the activity after several hours decaying to half value in about 28 minutes (see section 222). The rapid initial drop has been observed by
